The general Ideal Gas Law formula is
PV = nRT
For this scenario you want to solve for the number of moles (n) and then plug in the values that you know from the information given in the question
n = PV / RT
n = (5.8102 x 63.353) / (0.08206*527) = 8.5117 mol
meaning that there are 8.5117 moles of Radon (Rn) in the container